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1zun

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(New page: 200px<br /><applet load="1zun" size="450" color="white" frame="true" align="right" spinBox="true" caption="1zun, resolution 2.70&Aring;" /> '''Crystal Structure of...)
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[[Image:1zun.gif|left|200px]]<br /><applet load="1zun" size="350" color="white" frame="true" align="right" spinBox="true"
caption="1zun, resolution 2.70&Aring;" />
caption="1zun, resolution 2.70&Aring;" />
'''Crystal Structure of a GTP-Regulated ATP Sulfurylase Heterodimer from Pseudomonas syringae'''<br />
'''Crystal Structure of a GTP-Regulated ATP Sulfurylase Heterodimer from Pseudomonas syringae'''<br />
==Overview==
==Overview==
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Sulfate assimilation is a critical component of both primary and secondary, metabolism. An essential step in this pathway is the activation of sulfate, through adenylation by the enzyme ATP sulfurylase (ATPS), forming, adenosine 5'-phosphosulfate (APS). Proteobacterial ATPS overcomes this, energetically unfavorable reaction by associating with a regulatory G, protein, coupling the energy of GTP hydrolysis to APS formation. To, discover the molecular basis of this unusual role for a G protein, we, biochemically characterized and solved the X-ray crystal structure of a, complex between Pseudomonas syringae ATPS (CysD) and its associated, regulatory G protein (CysN). The structure of CysN*D shows the two, proteins in tight association; however, the nucleotides bound to each, subunit are spatially segregated. We provide evidence that conserved, switch motifs in the G domain of CysN allosterically mediate interactions, between the nucleotide binding sites. This structure suggests a molecular, mechanism by which conserved G domain architecture is used to, energetically link GTP turnover to the production of an essential, metabolite.
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Sulfate assimilation is a critical component of both primary and secondary metabolism. An essential step in this pathway is the activation of sulfate through adenylation by the enzyme ATP sulfurylase (ATPS), forming adenosine 5'-phosphosulfate (APS). Proteobacterial ATPS overcomes this energetically unfavorable reaction by associating with a regulatory G protein, coupling the energy of GTP hydrolysis to APS formation. To discover the molecular basis of this unusual role for a G protein, we biochemically characterized and solved the X-ray crystal structure of a complex between Pseudomonas syringae ATPS (CysD) and its associated regulatory G protein (CysN). The structure of CysN*D shows the two proteins in tight association; however, the nucleotides bound to each subunit are spatially segregated. We provide evidence that conserved switch motifs in the G domain of CysN allosterically mediate interactions between the nucleotide binding sites. This structure suggests a molecular mechanism by which conserved G domain architecture is used to energetically link GTP turnover to the production of an essential metabolite.
==About this Structure==
==About this Structure==
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1ZUN is a [http://en.wikipedia.org/wiki/Protein_complex Protein complex] structure of sequences from [http://en.wikipedia.org/wiki/Pseudomonas_syringae Pseudomonas syringae] and [http://en.wikipedia.org/wiki/Pseudomonas_syringae_pv._tomato_str._dc3000 Pseudomonas syringae pv. tomato str. dc3000] with MG, NA, GDP and AGS as [http://en.wikipedia.org/wiki/ligands ligands]. Active as [http://en.wikipedia.org/wiki/Sulfate_adenylyltransferase Sulfate adenylyltransferase], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=2.7.7.4 2.7.7.4] Full crystallographic information is available from [http://ispc.weizmann.ac.il/oca-bin/ocashort?id=1ZUN OCA].
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1ZUN is a [http://en.wikipedia.org/wiki/Protein_complex Protein complex] structure of sequences from [http://en.wikipedia.org/wiki/Pseudomonas_syringae Pseudomonas syringae] and [http://en.wikipedia.org/wiki/Pseudomonas_syringae_pv._tomato_str._dc3000 Pseudomonas syringae pv. tomato str. dc3000] with <scene name='pdbligand=MG:'>MG</scene>, <scene name='pdbligand=NA:'>NA</scene>, <scene name='pdbligand=GDP:'>GDP</scene> and <scene name='pdbligand=AGS:'>AGS</scene> as [http://en.wikipedia.org/wiki/ligands ligands]. Active as [http://en.wikipedia.org/wiki/Sulfate_adenylyltransferase Sulfate adenylyltransferase], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=2.7.7.4 2.7.7.4] Full crystallographic information is available from [http://oca.weizmann.ac.il/oca-bin/ocashort?id=1ZUN OCA].
==Reference==
==Reference==
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[[Category: Pseudomonas syringae pv. tomato str. dc3000]]
[[Category: Pseudomonas syringae pv. tomato str. dc3000]]
[[Category: Sulfate adenylyltransferase]]
[[Category: Sulfate adenylyltransferase]]
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[[Category: Berger, J.M.]]
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[[Category: Berger, J M.]]
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[[Category: Bertozzi, C.R.]]
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[[Category: Bertozzi, C R.]]
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[[Category: Hubbard, S.C.]]
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[[Category: Hubbard, S C.]]
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[[Category: Lee, D.H.]]
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[[Category: Lee, D H.]]
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[[Category: Mougous, J.D.]]
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[[Category: Mougous, J D.]]
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[[Category: Schelle, M.W.]]
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[[Category: Schelle, M W.]]
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[[Category: Vocadlo, D.J.]]
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[[Category: Vocadlo, D J.]]
[[Category: AGS]]
[[Category: AGS]]
[[Category: GDP]]
[[Category: GDP]]
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[[Category: switch domain]]
[[Category: switch domain]]
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''Page seeded by [http://ispc.weizmann.ac.il/oca OCA ] on Wed Nov 21 07:40:21 2007''
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Thu Feb 21 16:19:13 2008''

Revision as of 14:19, 21 February 2008


1zun, resolution 2.70Å

Drag the structure with the mouse to rotate

Crystal Structure of a GTP-Regulated ATP Sulfurylase Heterodimer from Pseudomonas syringae

Overview

Sulfate assimilation is a critical component of both primary and secondary metabolism. An essential step in this pathway is the activation of sulfate through adenylation by the enzyme ATP sulfurylase (ATPS), forming adenosine 5'-phosphosulfate (APS). Proteobacterial ATPS overcomes this energetically unfavorable reaction by associating with a regulatory G protein, coupling the energy of GTP hydrolysis to APS formation. To discover the molecular basis of this unusual role for a G protein, we biochemically characterized and solved the X-ray crystal structure of a complex between Pseudomonas syringae ATPS (CysD) and its associated regulatory G protein (CysN). The structure of CysN*D shows the two proteins in tight association; however, the nucleotides bound to each subunit are spatially segregated. We provide evidence that conserved switch motifs in the G domain of CysN allosterically mediate interactions between the nucleotide binding sites. This structure suggests a molecular mechanism by which conserved G domain architecture is used to energetically link GTP turnover to the production of an essential metabolite.

About this Structure

1ZUN is a Protein complex structure of sequences from Pseudomonas syringae and Pseudomonas syringae pv. tomato str. dc3000 with , , and as ligands. Active as Sulfate adenylyltransferase, with EC number 2.7.7.4 Full crystallographic information is available from OCA.

Reference

Molecular basis for G protein control of the prokaryotic ATP sulfurylase., Mougous JD, Lee DH, Hubbard SC, Schelle MW, Vocadlo DJ, Berger JM, Bertozzi CR, Mol Cell. 2006 Jan 6;21(1):109-22. PMID:16387658

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