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2bjm

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==Overview==
==Overview==
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Induced fit is a predominant phenomenon in protein-ligand interactions, yet it is invariably attributed without establishing the existence, let, alone the structure, of the initial, low-affinity encounter complex. We, determined the crystal structure of the encounter complex on the pathway, of ligand binding by IgE antibody SPE7. We show that this complex is, formed by a wide range of ligands that initially bind with identical, affinity. Nonspecific ligands rapidly dissociate, whereupon the antibody, isomerizes to a nonbinding isomer. Specific ligand complexes, however, slowly isomerize to give a high-affinity complex. This isomerization, involves backbone and side-chain rearrangements of up to 14 A and the, formation of specific hydrogen bonds. The postbinding conformational, switch, combined with the prebinding isomerization to an energetically, favorable nonbinding isomer, results in a "kinetic discrimination", mechanism that mediates selective binding, by a factor of >10(3), between, highly related ligands that initially bind with the same affinity. This, model may apply to proteins that bind multiple ligands in a specific, manner or other proteins that, although capable of binding many ligands, are activated by only a few.
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Induced fit is a predominant phenomenon in protein-ligand interactions, yet it is invariably attributed without establishing the existence, let alone the structure, of the initial, low-affinity encounter complex. We determined the crystal structure of the encounter complex on the pathway of ligand binding by IgE antibody SPE7. We show that this complex is formed by a wide range of ligands that initially bind with identical affinity. Nonspecific ligands rapidly dissociate, whereupon the antibody isomerizes to a nonbinding isomer. Specific ligand complexes, however, slowly isomerize to give a high-affinity complex. This isomerization involves backbone and side-chain rearrangements of up to 14 A and the formation of specific hydrogen bonds. The postbinding conformational switch, combined with the prebinding isomerization to an energetically favorable nonbinding isomer, results in a "kinetic discrimination" mechanism that mediates selective binding, by a factor of >10(3), between highly related ligands that initially bind with the same affinity. This model may apply to proteins that bind multiple ligands in a specific manner or other proteins that, although capable of binding many ligands, are activated by only a few.
==About this Structure==
==About this Structure==
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[[Category: Rattus rattus]]
[[Category: Rattus rattus]]
[[Category: Single protein]]
[[Category: Single protein]]
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[[Category: James, L.C.]]
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[[Category: James, L C.]]
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[[Category: Tawfik, D.S.]]
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[[Category: Tawfik, D S.]]
[[Category: ANF]]
[[Category: ANF]]
[[Category: antibody]]
[[Category: antibody]]
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[[Category: promiscuity]]
[[Category: promiscuity]]
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Sun Feb 3 10:24:56 2008''
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Thu Feb 21 16:38:32 2008''

Revision as of 14:38, 21 February 2008


2bjm, resolution 2.150Å

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SPE7:ANTHRONE COMPLEX

Overview

Induced fit is a predominant phenomenon in protein-ligand interactions, yet it is invariably attributed without establishing the existence, let alone the structure, of the initial, low-affinity encounter complex. We determined the crystal structure of the encounter complex on the pathway of ligand binding by IgE antibody SPE7. We show that this complex is formed by a wide range of ligands that initially bind with identical affinity. Nonspecific ligands rapidly dissociate, whereupon the antibody isomerizes to a nonbinding isomer. Specific ligand complexes, however, slowly isomerize to give a high-affinity complex. This isomerization involves backbone and side-chain rearrangements of up to 14 A and the formation of specific hydrogen bonds. The postbinding conformational switch, combined with the prebinding isomerization to an energetically favorable nonbinding isomer, results in a "kinetic discrimination" mechanism that mediates selective binding, by a factor of >10(3), between highly related ligands that initially bind with the same affinity. This model may apply to proteins that bind multiple ligands in a specific manner or other proteins that, although capable of binding many ligands, are activated by only a few.

About this Structure

2BJM is a Single protein structure of sequence from Rattus rattus with as ligand. Known structural/functional Site: . Full crystallographic information is available from OCA.

Reference

Structure and kinetics of a transient antibody binding intermediate reveal a kinetic discrimination mechanism in antigen recognition., James LC, Tawfik DS, Proc Natl Acad Sci U S A. 2005 Sep 6;102(36):12730-5. Epub 2005 Aug 29. PMID:16129832

Page seeded by OCA on Thu Feb 21 16:38:32 2008

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