1l2u

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(New page: 200px<br /><applet load="1l2u" size="450" color="white" frame="true" align="right" spinBox="true" caption="1l2u, resolution 2.5&Aring;" /> '''Orotidine 5'-monophos...)
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caption="1l2u, resolution 2.5&Aring;" />
'''Orotidine 5'-monophosphate decarboxylase from E. coli'''<br />
'''Orotidine 5'-monophosphate decarboxylase from E. coli'''<br />
==Overview==
==Overview==
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Orotidine 5'-monophosphate decarboxylase (ODCase) catalyses the, decarboxylation of orotidine 5'-monophosphate to uridine 5'-monophosphate, (UMP). We have earlier determined the structure of ODCase from Escherichia, coli complexed with the inhibitor, 1-(5'-phospho-beta-d-ribofuranosyl)barbituric acid (BMP); here we present, the 2.5 A structure of the uncomplexed apo enzyme, determined from twinned, crystals. A structural analysis and comparison of the two structures of, the E. coli enzyme show that binding of the inhibitor is accompanied by, significant domain movements of approximately 12 degrees around a hinge, that crosses the active site. Hence, the ODCase dimer, which contains two, active sites, may be divided in three domains: a central domain that is, fixed, and two lids which independently move 12 degrees upon binding., Corresponding analyses, presented herein, of the two Saccharomyces, cerevisiae ODCase structures (with and without BMP) and the, Methanobacterium thermoautotrophicum ODCase structures (with and without, 6-aza UMP) show very similar, but somewhat smaller domain movements. The, domain movements seem to be initiated by the phosphoryl binding to the, enzyme and can explain why the binding of the phosphoryl group is, essential for the catalytic function.
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Orotidine 5'-monophosphate decarboxylase (ODCase) catalyses the decarboxylation of orotidine 5'-monophosphate to uridine 5'-monophosphate (UMP). We have earlier determined the structure of ODCase from Escherichia coli complexed with the inhibitor 1-(5'-phospho-beta-d-ribofuranosyl)barbituric acid (BMP); here we present the 2.5 A structure of the uncomplexed apo enzyme, determined from twinned crystals. A structural analysis and comparison of the two structures of the E. coli enzyme show that binding of the inhibitor is accompanied by significant domain movements of approximately 12 degrees around a hinge that crosses the active site. Hence, the ODCase dimer, which contains two active sites, may be divided in three domains: a central domain that is fixed, and two lids which independently move 12 degrees upon binding. Corresponding analyses, presented herein, of the two Saccharomyces cerevisiae ODCase structures (with and without BMP) and the Methanobacterium thermoautotrophicum ODCase structures (with and without 6-aza UMP) show very similar, but somewhat smaller domain movements. The domain movements seem to be initiated by the phosphoryl binding to the enzyme and can explain why the binding of the phosphoryl group is essential for the catalytic function.
==About this Structure==
==About this Structure==
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1L2U is a [http://en.wikipedia.org/wiki/Single_protein Single protein] structure of sequence from [http://en.wikipedia.org/wiki/Escherichia_coli Escherichia coli]. Active as [http://en.wikipedia.org/wiki/Orotidine-5'-phosphate_decarboxylase Orotidine-5'-phosphate decarboxylase], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=4.1.1.23 4.1.1.23] Full crystallographic information is available from [http://ispc.weizmann.ac.il/oca-bin/ocashort?id=1L2U OCA].
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1L2U is a [http://en.wikipedia.org/wiki/Single_protein Single protein] structure of sequence from [http://en.wikipedia.org/wiki/Escherichia_coli Escherichia coli]. Active as [http://en.wikipedia.org/wiki/Orotidine-5'-phosphate_decarboxylase Orotidine-5'-phosphate decarboxylase], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=4.1.1.23 4.1.1.23] Full crystallographic information is available from [http://oca.weizmann.ac.il/oca-bin/ocashort?id=1L2U OCA].
==Reference==
==Reference==
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[[Category: Single protein]]
[[Category: Single protein]]
[[Category: Harris, P.]]
[[Category: Harris, P.]]
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[[Category: Jensen, K.F.]]
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[[Category: Jensen, K F.]]
[[Category: Larsen, S.]]
[[Category: Larsen, S.]]
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[[Category: Poulsen, J.C.]]
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[[Category: Poulsen, J C.]]
[[Category: beta-alpha-barrel]]
[[Category: beta-alpha-barrel]]
[[Category: homodimer]]
[[Category: homodimer]]
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[[Category: x-ray diffraction]]
[[Category: x-ray diffraction]]
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''Page seeded by [http://ispc.weizmann.ac.il/oca OCA ] on Tue Nov 20 20:12:03 2007''
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Thu Feb 21 13:40:43 2008''

Revision as of 11:40, 21 February 2008


1l2u, resolution 2.5Å

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Orotidine 5'-monophosphate decarboxylase from E. coli

Overview

Orotidine 5'-monophosphate decarboxylase (ODCase) catalyses the decarboxylation of orotidine 5'-monophosphate to uridine 5'-monophosphate (UMP). We have earlier determined the structure of ODCase from Escherichia coli complexed with the inhibitor 1-(5'-phospho-beta-d-ribofuranosyl)barbituric acid (BMP); here we present the 2.5 A structure of the uncomplexed apo enzyme, determined from twinned crystals. A structural analysis and comparison of the two structures of the E. coli enzyme show that binding of the inhibitor is accompanied by significant domain movements of approximately 12 degrees around a hinge that crosses the active site. Hence, the ODCase dimer, which contains two active sites, may be divided in three domains: a central domain that is fixed, and two lids which independently move 12 degrees upon binding. Corresponding analyses, presented herein, of the two Saccharomyces cerevisiae ODCase structures (with and without BMP) and the Methanobacterium thermoautotrophicum ODCase structures (with and without 6-aza UMP) show very similar, but somewhat smaller domain movements. The domain movements seem to be initiated by the phosphoryl binding to the enzyme and can explain why the binding of the phosphoryl group is essential for the catalytic function.

About this Structure

1L2U is a Single protein structure of sequence from Escherichia coli. Active as Orotidine-5'-phosphate decarboxylase, with EC number 4.1.1.23 Full crystallographic information is available from OCA.

Reference

Substrate binding induces domain movements in orotidine 5'-monophosphate decarboxylase., Harris P, Poulsen JC, Jensen KF, Larsen S, J Mol Biol. 2002 May 10;318(4):1019-29. PMID:12054799

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