1loy

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|PDB= 1loy |SIZE=350|CAPTION= <scene name='initialview01'>1loy</scene>, resolution 1.55&Aring;
|PDB= 1loy |SIZE=350|CAPTION= <scene name='initialview01'>1loy</scene>, resolution 1.55&Aring;
|SITE=
|SITE=
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|LIGAND= <scene name='pdbligand=CA:CALCIUM+ION'>CA</scene> and <scene name='pdbligand=3GP:GUANOSINE-3&#39;-MONOPHOSPHATE'>3GP</scene>
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|LIGAND= <scene name='pdbligand=3GP:GUANOSINE-3&#39;-MONOPHOSPHATE'>3GP</scene>, <scene name='pdbligand=CA:CALCIUM+ION'>CA</scene>
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|ACTIVITY= [http://en.wikipedia.org/wiki/Ribonuclease_T(1) Ribonuclease T(1)], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=3.1.27.3 3.1.27.3]
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|ACTIVITY= <span class='plainlinks'>[http://en.wikipedia.org/wiki/Ribonuclease_T(1) Ribonuclease T(1)], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=3.1.27.3 3.1.27.3] </span>
|GENE=
|GENE=
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|DOMAIN=
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|RELATEDENTRY=[[1rga|1RGA]], [[1rls|1RLS]], [[1lov|1LOV]], [[1low|1LOW]]
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|RESOURCES=<span class='plainlinks'>[http://oca.weizmann.ac.il/oca-docs/fgij/fg.htm?mol=1loy FirstGlance], [http://oca.weizmann.ac.il/oca-bin/ocaids?id=1loy OCA], [http://www.ebi.ac.uk/pdbsum/1loy PDBsum], [http://www.rcsb.org/pdb/explore.do?structureId=1loy RCSB]</span>
}}
}}
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[[Category: Mignon, P.]]
[[Category: Mignon, P.]]
[[Category: Steyaert, J.]]
[[Category: Steyaert, J.]]
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[[Category: 3GP]]
 
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[[Category: CA]]
 
[[Category: ab initio calculation]]
[[Category: ab initio calculation]]
[[Category: catalytic dyad]]
[[Category: catalytic dyad]]
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[[Category: rnase]]
[[Category: rnase]]
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Sun Mar 23 12:39:21 2008''
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Sun Mar 30 22:05:31 2008''

Revision as of 19:05, 30 March 2008


PDB ID 1loy

Drag the structure with the mouse to rotate
, resolution 1.55Å
Ligands: ,
Activity: Ribonuclease T(1), with EC number 3.1.27.3
Related: 1RGA, 1RLS, 1LOV, 1LOW


Resources: FirstGlance, OCA, PDBsum, RCSB
Coordinates: save as pdb, mmCIF, xml



X-ray structure of the H40A/E58A mutant of Ribonuclease T1 complexed with 3'-guanosine monophosphate


Overview

Ribonucleases (RNases) catalyze the cleavage of the phosphodiester bond in RNA up to 10(15)-fold, as compared with the uncatalyzed reaction. High resolution crystal structures of these enzymes in complex with 3'-mononucleotide substrates demonstrate the accommodation of the nucleophilic 2'-OH group in a binding pocket comprising the catalytic base (glutamate or histidine) and a charged hydrogen bond donor (lysine or histidine). Ab initio quantum chemical calculations performed on such Michaelis complexes of the mammalian RNase A (EC ) and the microbial RNase T(1) (EC ) show negative charge build up on the 2'-oxygen upon substrate binding. The increased nucleophilicity results from stronger hydrogen bonding to the catalytic base, which is mediated by a hydrogen bond from the charged donor. This hitherto unrecognized catalytic dyad in ribonucleases constitutes a general mechanism for nucleophile activation in both enzymic and RNA-catalyzed phosphoryl transfer reactions.

About this Structure

1LOY is a Single protein structure of sequence from Aspergillus oryzae. Full crystallographic information is available from OCA.

Reference

A nucleophile activation dyad in ribonucleases. A combined X-ray crystallographic/ab initio quantum chemical study., Mignon P, Steyaert J, Loris R, Geerlings P, Loverix S, J Biol Chem. 2002 Sep 27;277(39):36770-4. Epub 2002 Jul 16. PMID:12122018

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