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1qt4

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[[Image:1qt4.jpg|left|200px]]
[[Image:1qt4.jpg|left|200px]]
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{{Structure
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<!--
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|PDB= 1qt4 |SIZE=350|CAPTION= <scene name='initialview01'>1qt4</scene>, resolution 2.1&Aring;
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The line below this paragraph, containing "STRUCTURE_1qt4", creates the "Structure Box" on the page.
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|SITE=
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You may change the PDB parameter (which sets the PDB file loaded into the applet)
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|LIGAND= <scene name='pdbligand=BME:BETA-MERCAPTOETHANOL'>BME</scene>, <scene name='pdbligand=CL:CHLORIDE+ION'>CL</scene>
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or the SCENE parameter (which sets the initial scene displayed when the page is loaded),
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|ACTIVITY= <span class='plainlinks'>[http://en.wikipedia.org/wiki/Lysozyme Lysozyme], with EC number [http://www.brenda-enzymes.info/php/result_flat.php4?ecno=3.2.1.17 3.2.1.17] </span>
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or leave the SCENE parameter empty for the default display.
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|GENE=
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-->
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|DOMAIN=
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{{STRUCTURE_1qt4| PDB=1qt4 | SCENE= }}
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|RELATEDENTRY=[[1qtv|1QTV]], [[1qtz|1QTZ]], [[1qt3|1QT3]], [[1qt5|1QT5]], [[1qt6|1QT6]], [[1qt7|1QT7]], [[1qt8|1QT8]]
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|RESOURCES=<span class='plainlinks'>[http://oca.weizmann.ac.il/oca-docs/fgij/fg.htm?mol=1qt4 FirstGlance], [http://oca.weizmann.ac.il/oca-bin/ocaids?id=1qt4 OCA], [http://www.ebi.ac.uk/pdbsum/1qt4 PDBsum], [http://www.rcsb.org/pdb/explore.do?structureId=1qt4 RCSB]</span>
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}}
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'''T26Q MUTANT OF T4 LYSOZYME'''
'''T26Q MUTANT OF T4 LYSOZYME'''
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[[Category: Matthews, B W.]]
[[Category: Matthews, B W.]]
[[Category: Weaver, L H.]]
[[Category: Weaver, L H.]]
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[[Category: hydrolase]]
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[[Category: Hydrolase]]
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Sat May 3 06:40:38 2008''
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''Page seeded by [http://oca.weizmann.ac.il/oca OCA ] on Sun Mar 30 23:18:39 2008''
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Revision as of 03:40, 3 May 2008

Template:STRUCTURE 1qt4

T26Q MUTANT OF T4 LYSOZYME


Overview

In contrast to hen egg-white lysozyme, which retains the beta-configuration of the substrate in the product, T4 lysozyme (T4L) is an inverting glycosidase. The substitution Thr-26 --> His, however, converts T4L from an inverting to a retaining enzyme. It is shown here that the Thr-26 --> His mutant is also a transglycosidase. Indeed, the transglycosylation reaction can be more effective than hydrolysis. In contrast, wild-type T4L has no detectable transglycosidase activity. The results support the prior hypothesis that catalysis by the Thr-26 --> His mutant proceeds via a covalent intermediate. Further mutations (Glu-11 --> His, Asp-20 --> Cys) of the T26H mutant lysozyme indicate that the catalytic mechanism of this mutant requires Glu-11 as a general acid but Asp-20 is not essential. The results help provide an overall rationalization for the activity of glycosidases, in which a highly conserved acid group (Glu-11 in T4L, Glu-35 in hen egg-white lysozyme) on the beta-side of the substrate acts as a proton donor, whereas alterations in the placement and chemical identity of residues on the alpha-side of the substrate can lead to catalysis with or without retention of the configuration, to transglycosidase activity, or to the formation of a stable enzyme-substrate adduct.

About this Structure

1QT4 is a Single protein structure of sequence from Enterobacteria phage t4. Full crystallographic information is available from OCA.

Reference

Structural basis of the conversion of T4 lysozyme into a transglycosidase by reengineering the active site., Kuroki R, Weaver LH, Matthews BW, Proc Natl Acad Sci U S A. 1999 Aug 3;96(16):8949-54. PMID:10430876 Page seeded by OCA on Sat May 3 06:40:38 2008

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