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3bto

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Revision as of 15:40, 30 October 2007 by OCA (Talk | contribs)
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3bto, resolution 1.66Å

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HORSE LIVER ALCOHOL DEHYDROGENASE COMPLEXED TO NADH AND (1S,3S)3-BUTYLTHIOLANE 1-OXIDE

Overview

Thiolane 1-oxides are analogs of the carbonyl substrates that bind to the, alcohol dehydrogenase-NADH complex and are potent uncompetitive inhibitors, against alcohol [Chadha, V. K., et al. (1985) J. Med. Chem. 28, 36-40]., The four stereoisomers of 3-butylthiolane 1-oxide (BTO) were separated by, chiral phase chromatography. CD and 1H-NMR spectra identified the, enantiomeric pairs. 1H-NMR chemical shifts were assigned on the basis of, COSY spectra of both diastereoisomers and confirmed by HMQC spectra., Coupling constants were determined through one-dimensional decoupling, experiments. NMR with chiral shift reagents, Eu(hfc)3 [europium tris, [3-[(heptafluoropropyl)hydroxymethylene]-(+)-camphorate]] or, (R)-(-)-N-(3,5-dinitrobenzoyl)-alpha-methylbenzylamine, determined that, the most ... [(full description)]

About this Structure

3BTO is a [Single protein] structure of sequence from [Equus caballus] with ZN, NAD and SSB as [ligands]. Active as [Alcohol dehydrogenase], with EC number [1.1.1.1]. Structure known Active Site: NAD. Full crystallographic information is available from [OCA].

Reference

Flexibility of liver alcohol dehydrogenase in stereoselective binding of 3-butylthiolane 1-oxides., Cho H, Ramaswamy S, Plapp BV, Biochemistry. 1997 Jan 14;36(2):382-9. PMID:9003191

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